Ramanand Sagar's was a Tulsidas-only based project, whereas Ananda Sagar's was a khichri of everybody - Tulsidas, Kamban, Krittivas, Adhyatma, et al. Dunno which one would be deemed better, but that's the difference b/w the 2. There was also the difference in ambiance.
As for the actors, I think who was better, aside from being subjective, varied according to the roles. Like the old Shurpanakha was more authentic, but the the old Indrajit was way too hyper
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